Single cell imaging of Bruton's Tyrosine Kinase using an irreversible inhibitor

نویسندگان

  • Anna Turetsky
  • Eunha Kim
  • Rainer H. Kohler
  • Miles A. Miller
  • Ralph Weissleder
چکیده

A number of Bruton's tyrosine kinase (BTK) inhibitors are currently in development, yet it has been difficult to visualize BTK expression and pharmacological inhibition in vivo in real time. We synthesized a fluorescent, irreversible BTK binder based on the drug Ibrutinib and characterized its behavior in cells and in vivo. We show a 200 nM affinity of the imaging agent, high selectivity, and irreversible binding to its target following initial washout, resulting in surprisingly high target-to-background ratios. In vivo, the imaging agent rapidly distributed to BTK expressing tumor cells, but also to BTK-positive tumor-associated host cells.

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عنوان ژورنال:

دوره 4  شماره 

صفحات  -

تاریخ انتشار 2014